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Renin Angiotensin Mechanism.

Enzyme Inhibition.

 

Introduction:

  • Enzymes are the organic biological catalysts, which speed up the rate of biochemical reactions without undergoing any change.

  • They are  highly selective catalysts that greatly accelerate both the rate and specificity of metabolic reactions.

  • Many types of molecules exist which are capable of obstructing the activity of an individual enzyme.

  • An inhibitor is any molecule that acts directly on an enzyme to reduce its catalytic rate.

  • Some enzyme inhibitors are normal body metabolites that inhibit a particular enzyme while other inhibitors may be foreign substances, such as drugs or toxins.

  • The inhibition may be a part of the normal metabolic control of a pathway, a diseased condition or either a therapeutic measure.

  • The effect of enzyme inhibition could be either therapeutic or, at the other extreme, dangerous.

  • Enzyme inhibition is of two main types:

    • Irreversible Inhibition

    • Reversible Inhibition

      • Competitive reversible inhibition and

      • Non-competitive reversible inhibition.


Irreversible Inhibition.

  • Irreversible inhibitors bind to the enzyme and inactivate it.

  • Inhibitors that bind irreversibly to an enzyme frequently form a covalent bond to an amino acid residue at or near the active site, inactivating the enzyme permanently.

  • Susceptible amino acid residues include Ser and Cys residues which have reactive –OH and –SH groups, respectively.

  • Some nonspecific inhibitors may cause physical or chemical change to the enzyme structure e.g. denaturation.

  • e.g 

    • Organophosphorus compounds (Insecticides), covalently bond the active site of the enzyme acetylcholinesterase, irreversibly inhibiting the enzyme.

    • Penicillin inhibits the glycopeptide transpeptidase enzyme, which forms cross-links in the bacterial cell wall, irreversibly by covalently attaching to a “Ser” residue in the enzyme's active site.

Reversible Inhibition.

  • Reversible inhibition can be overcome by removing the inhibitor from the enzyme.

  • Reversible enzyme inhibitors can be classified as either competitive or noncompetitive, and can be distinguished via a Lineweaver–Burk plot.

Competitive Inhibitors:

  • Competitive inhibitors compete with the substrate for the active site of the enzyme and form an enzyme–substrate complex.

  • A competitive inhibitor typically has close structural similarities to the normal substrate for the enzyme. Thus it competes with substrate molecules to bind to the active site.

  • As the enzyme can bind either a substrate or an inhibitor, but not both at the same time; binding to the inhibitor inhibits its activity.

  • The competitive inhibitor binds reversibly to the active site.

  • At high substrate concentrations the action of a competitive inhibitor is reversed because a sufficiently high substrate concentration will successfully compete out the inhibitor molecule in binding to the active site.

  • Many drugs work by mimicking the structure of the substrate of a target enzyme, and hence act as competitive inhibitors of the enzyme.

    • e.g. Sulfonamides and PABA.

Non- competitive Inhibitors:

  • Non- competitive inhibitors bind to the enzyme or the enzyme–substrate complex at a site different from the active site, hence decreasing the activity of the enzyme.

  • A noncompetitive inhibitor binds reversibly at a site other than the active site and causes a change in the overall 3-D shape of the enzyme that leads to a decrease in the activity.

  • Since the inhibitor binds at a different site from the substrate, the enzyme may bind the inhibitor, the substrate or both the inhibitor and substrate together.

  • The effects of a non-competitive inhibitor cannot be overcome by increasing the substrate concentration, so there is a decrease in Vmax.

    • e.g.  action of pepstatin (A protease inhibitor) on the enzyme renin.

Commonly Asked Question.

  1. Write a short note on Enzyme Inhibition.

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